Spiewanowski, Maciek2; Etches, Adam2; Madsen, Lars Bojer2
1 Department of Physics and Astronomy, Science and Technology, Aarhus University2 Department of Physics and Astronomy, Science and Technology, Aarhus University
We investigate the eect on high-order harmonic generation of the distortion of molecular orbitals by the driving laser eld. Calculations for high-order harmonic generation including orbital distortion are performed for N2 (high polarizability). Our results allow us to suggest that field-distortion is the reason why the two-center interference minimum has never been observed experimentally in N2. We propose experimental parameters which should allow an observation of the two-center interference minimum. Calculations for CO2 (low polarizability) further validate the theory by revealing the survival of the minimum in the high-order harmonic spectra. This is in agreement with experiment.
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International Conference on Attosecond Physics 2013